I've ridden in my coworkers 2015 CTS many, many times. Personally I feel that it is more "floaty" feeling in its suspension. It is just in how smooth everything is. It's quite a bit more luxurious. The bigger V8 motor though, you can't beat a V8 growl and raw power... it is by far cooler in that aspect.
The ATS I own is bit rougher, chirpier, responsive, and honestly I think quicker (up to) high speeds. (CTS-V has a hellova lot more motor if you go top-end, and the ATS simply can't keep up)
But as a 2.0T owner, using it to commute in Houston traffic, it's LOTS of fun to cruise in. Good gas mileage too!
Remember, the back seat it tiny. Kids, briefcase, coats, small things. Not really good for adults. (but you can fit if needed)
To me, driving the ATS feels like a more luxurious 4-door Lotus with an air conditioner and radio, on a budget.
I do intend to finish tweaking my ATS for high power (new turbo, all internals, cams, intake/exhaust), high performance suspension, brakes, and wider tires. (probably will need to flare the fenders... eventually)
When I do all that, it will be a high $ ride, but I bet it scares the rest of the hair off my head on the track. haha